Sorption and ion exchange have been examined as suitable direct lithium extraction (DLE) techniques. For the DLE technique, sorbents are needed that selectively bind lithium. Commercially available sorbents, however, have advantages and disadvantages in different processing lines and in dependence on the physicochemical parameters during extraction. In the joint UnLimited project, different sorbents beyond Mn-oxide are tested at lab scale, i.e., zeolite and Li-Fe-phosphate.